Iron-containing atmospheric aerosols in the Chernobyl fallout

V. Rusanov; V. Gushterov; H. Winkler; A. X. Trautwein

doi:10.1007/s10751-006-9331-4

Iron-containing atmospheric aerosols in the Chernobyl fallout

V. Rusanov, V. Gushterov^*, H. Winkler, A. X. Trautwein

^*Korrespondierende/r Autor/-in für diese Arbeit

Institut für Physik

University of Sofia

Abstract

Mössbauer spectroscopy was applied to determine the composition and the iron concentration in the atmospheric aerosols contaminated in Sofia, Bulgaria after the Chernobyl accident. The results confirm the major conclusion of the Kopcewiczs for Poland, i.e. that in the initial filters, collected during the contaminating fallout (30.04-05.05.1986), the iron concentration was highest, 3.69 μg/m³ and that magnetite Fe₃O₄ was present. For the following days a change in the chemical composition including the presence of α-Fe₂O₃, α-FeOOH and γ-FeOOH as well as the absence of magnetite, was detected. Input of industrial iron contamination was negligible since the nearby steel plant had worked at minimum power due to official holidays. Unfortunately, Mössbauer spectroscopy studies only, do not allow a definite conclusion about an increase of the isotope abundance of ⁵⁷Fe in the Chernobyl fallout.

Originalsprache	Englisch
Zeitschrift	Hyperfine Interactions
Jahrgang	166
Ausgabenummer	1-4
Seiten (von - bis)	625-630
Seitenumfang	6
ISSN	0304-3843
DOIs	https://doi.org/10.1007/s10751-006-9331-4
Publikationsstatus	Veröffentlicht - 01.11.2005

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Acknowledgements The authors are indebted to Mr V. Mavrodiev for providing the filters. Thanks are due to the Alexander von Humboldt Foundation, special program Stability Pact for South Eastern Europe (V. R. and A. X. T.).

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10.1007/s10751-006-9331-4

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title = "Iron-containing atmospheric aerosols in the Chernobyl fallout",

abstract = "M{\"o}ssbauer spectroscopy was applied to determine the composition and the iron concentration in the atmospheric aerosols contaminated in Sofia, Bulgaria after the Chernobyl accident. The results confirm the major conclusion of the Kopcewiczs for Poland, i.e. that in the initial filters, collected during the contaminating fallout (30.04-05.05.1986), the iron concentration was highest, 3.69 μg/m3 and that magnetite Fe3O4 was present. For the following days a change in the chemical composition including the presence of α-Fe2O3, α-FeOOH and γ-FeOOH as well as the absence of magnetite, was detected. Input of industrial iron contamination was negligible since the nearby steel plant had worked at minimum power due to official holidays. Unfortunately, M{\"o}ssbauer spectroscopy studies only, do not allow a definite conclusion about an increase of the isotope abundance of 57Fe in the Chernobyl fallout.",

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T1 - Iron-containing atmospheric aerosols in the Chernobyl fallout

AU - Rusanov, V.

AU - Gushterov, V.

AU - Winkler, H.

AU - Trautwein, A. X.

PY - 2005/11/1

Y1 - 2005/11/1

N2 - Mössbauer spectroscopy was applied to determine the composition and the iron concentration in the atmospheric aerosols contaminated in Sofia, Bulgaria after the Chernobyl accident. The results confirm the major conclusion of the Kopcewiczs for Poland, i.e. that in the initial filters, collected during the contaminating fallout (30.04-05.05.1986), the iron concentration was highest, 3.69 μg/m3 and that magnetite Fe3O4 was present. For the following days a change in the chemical composition including the presence of α-Fe2O3, α-FeOOH and γ-FeOOH as well as the absence of magnetite, was detected. Input of industrial iron contamination was negligible since the nearby steel plant had worked at minimum power due to official holidays. Unfortunately, Mössbauer spectroscopy studies only, do not allow a definite conclusion about an increase of the isotope abundance of 57Fe in the Chernobyl fallout.

AB - Mössbauer spectroscopy was applied to determine the composition and the iron concentration in the atmospheric aerosols contaminated in Sofia, Bulgaria after the Chernobyl accident. The results confirm the major conclusion of the Kopcewiczs for Poland, i.e. that in the initial filters, collected during the contaminating fallout (30.04-05.05.1986), the iron concentration was highest, 3.69 μg/m3 and that magnetite Fe3O4 was present. For the following days a change in the chemical composition including the presence of α-Fe2O3, α-FeOOH and γ-FeOOH as well as the absence of magnetite, was detected. Input of industrial iron contamination was negligible since the nearby steel plant had worked at minimum power due to official holidays. Unfortunately, Mössbauer spectroscopy studies only, do not allow a definite conclusion about an increase of the isotope abundance of 57Fe in the Chernobyl fallout.

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JO - Hyperfine Interactions

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Iron-containing atmospheric aerosols in the Chernobyl fallout

Abstract

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